Loose

Furtado's third album, Loose, was released in June 2006. It was named partly after the spontaneous, creative decisions she faced while creating the album and also for the band TLC, who she said she admires for "taking back their sexuality, showing they were complete women." Four lead singles were released in different regions of the world: the Spanish reggaeton-influenced "No Hay Igual" (featuring Calle 13), the hip-hop "Promiscuous" (featuring Timbaland), the latin "Te Busque" (featuring Juanes) and the pop "Maneater". For the first time, Furtado worked with a variety of record producers and followed a more collaborative approach in creating the album. The album, mostly produced by Timbaland, showed her experimenting with a more R&B–hip hop sound and the "surreal, theatrical elements of '80s music". She has categorized the album's sound as punk-hop, which she describes as "this modern, poppy, spooky music" and stated that "there's a mysterious, after-midnight vibe to it that's extremely visceral". She attributed the youthful sound of the album to the presence of her two-year old daughter.

Furtado also wanted the album to sound more like her demo tapes which she prefers over her finished albums. She recalls, "The cool thing is we did the mixes as we went. The whole album is a board mix theoretically. We didn't bring in the fancy mixer at the end". During the album's creation, she listened to several electro and hard rock musicians including System of a Down and Death from Above 1979 who influenced the rock sounds present on the album and the "coughing, laughing, distorted bass lines" which were kept in the songs deliberately.

Loose became the most successful album of Furtado's career, reaching number-one in several countries including the United States and Canada and producing the hit singles, "Promiscuous" and "Maneater", which became the most successful songs of her career, reaching number-one in many countries. The album received generally positive reviews from critics, with some citing the "revitalising" effect of Timbaland on Furtado's music, and others calling it "slick, smart and surprising."

In June 2006, in an interview with Genre magazine, when asked if she had "ever felt an attraction to women", Furtado replied "Absolutely. Women are beautiful and sexy." She also said the idea that everyone was inherently bisexual made sense to her and agreed with Kurt Cobain's statement that "everyone is gay" from Nirvana's "All Apologies". This was considered by some to be an admission of bisexuality , but in August 2006, she confirmed that she was "straight, but very open-minded". She commented that she was slightly embarrassed by the quotes and stated, "I guess I was humouring the journalist a little and I was reading a book about Chinese medicine, and we went off on a tangent."

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